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Charge carrier transport and photogeneration in P3HT: This article reviews the charge transport and photogeneration in bulk-heterojunction solar cells made from blend films of regioregular poly 3-hexylthiophene RR-P3HT and methano-fullerene PCBM. This significant increase of the hole mobility balances the electron and hole mobilities in a photovoltaic blend in turn reducing space- charge formation, and this is the most important factor for the strong enhancement of the photovoltaic efficiency compared to an as cast, that is, non-annealed device.
PCBM blends in combination with a field- and temperature-independent charge carrier generation and greatly reduced non-geminate recombination explains the large quantum efficiencies mea-sured in P3HT: Thus photocarrier generation on photoexcitation of the conjugated rigid However, upon illumination only two symmetric switching peaks appeared during the same J-V measurement.
The similar difference between dark and illumination were also obtained in capacitance-voltage characteristics.
These results showed the strong influence of internal fields by photogenerated carriers , which modifies the polarization reversal process of ferroelectric layer. The gradual shift of the polarization reversal with increase of illumination intensity is assigned to the space- charge field of trapped electrons. Photo-generated carriers lose energy during extraction from polymer-fullerene solar cells.
In photovoltaic devices, the photo-generated charge carriers are typically assumed to be in thermal equilibrium with the lattice. In conventional materials, this assumption is experimentally justified as carrier thermalization completes before any significant carrier transport has occurred.
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